杨帆课题组介绍
| 课题组长 |
| 研究介绍 |
杨帆研究员主要从事表界面动态催化研究,面向催化探针小分子(CO, CO2, H2, O2, H2O)的催化活化与定向转化(特别是CO/CO2的选择性转化),通过发展模型催化体系和基于扫描探针与红外的原位动态表征方法,解析反应条件下催化活性位动态结构及其对上述探针分子的吸附、活化机制,在原子、分子尺度定量描述多相催化动态构-效关系。近五年来以通讯作者在Nat. Catal.,J. Am. Chem. Soc.,Nat. Commun.等期刊发表论文三十多篇。获Gordon Research Conferences Young Investigator Award、基金委青年科学基金A类资助,作为核心成员获2017年全国创新争先奖牌。现任Chinese Journal of Catalysis (催化学报)等多本期刊编委,中国化学会表面物理化学专业委员会与世界顶尖科学家论坛青年科学家委员会委员,中国微米纳米技术学会微纳米测量与仪器分会理事。曾任中国化学会催化专业委员会秘书长,参与组织第十六届国际催化大会,工况催化表征会议(Operando VIII)等重要国际学术会议。主持或参与承担自然科学基金委面上/重点/集成项目,科技部国家重点研发计划,中科院先导项目,中科院-美国能源部交流合作项目等基础科研项目。 本课题组长期诚聘副研究员、助理研究员、博士后、硕博连读研究生,待遇优厚,工作环境优越,欢迎有志于在催化化学、表面科学等领域开展最前沿研究的学生学者加入!有意者请直接与杨帆邮件联系。 |
| 发表文章 |
1. Shao, W.; Ning, Y.; Liao, W.; Yu, X.; Zhu, B.; Liu, Y.; Zhang, Y.; Yu, L.; Liu, Q.; Chen, H.; Zhang, L.; Meng, W.; Wang, X.; Chen, M.; Fu, Q.; Liu, P.; Yang, F.*; Bao, X., Continuity of reaction kinetics across the pressure and materials gaps in CO oxidation on FeO–Pt interfaces. Nature Catalysis 2026,9 (1), 37–47.
2. Sun, Z.; Wang, K.; Chen, C.; Chen, M.; Chen, X.; Yang, F.*; Liu, Y.; He, H.; Cao, Y., Inverse Al-ZrO2/Cu catalysts enable the on-purpose production of separable para-xylene and ethylene glycol from PET wastes. J. Am. Chem. Soc. 2026,148, 11822–11833.
3. Li, J.; Lai, Y.; Zhang, J.; Xu, S.; Wang, S.; Fan, W.; Yan, W.; Liu, Z.; Meng, X.; Yang, F.; Xiao, F.-S., Regulation of Al sites in AEI framework from different zeolite precursors for selective catalytic reduction of NOx with methane. J. Catal. 2026,454, 116660.
4. Hu, W.; Ma, L.; Ni, X.; Zou, Z.; Yang, F.; Wen, K.; Yang, H., Defect engineering of CuO nanosheets enables stable Cuδ+ for highly selective and productive CO2-to-C2+ electroreduction. Chem. Eng. J. 2026,541, 177334.
5. Zhu, B. W.; Huang, Y. X.; Lv, J. Y.; Huang, W. G.; Lian, Z.; Ouyang, R. H.; Yang, F.*, Dynamic evolution and transformation of copper oxides on Cu(111). J. Phys. Chem. C 2025,129 (29), 13497–13504.
6. Zhang, H.; Lou, S.; Yang, F..; Fan, K.; Gu, Z.; Li, W.; Chen, Y.; Gan, Y.; Ma, L.; Wang, G.; Yang, H., Imidazolium salt-functionalized Cu2O@SiO2 catalysts for integrated CO2 capture and electroreduction to multi-carbon products in acidic electrolytes. Chem. Eng. J. 2025,522, 167793.
7. Shao, W.-P.; Ling, Y.; Peng, H.; Luo, J.; Cao, Y.; Ran, Y.; Cai, J.; Lv, J.; Zhu, B.; Liu, Y.; Chen, Y.; Li, N.; Jiao, F.; Chen, H.; Zhu, Y.; Ou, X.; Wang, Y.; Wöll, C.; Fu, Q.; Pan, X.; Hu, P.; Li, W.-X.; Liu, Z.; Bao, X.; Yang, F.*, Ion irradiation-induced coordinatively unsaturated Zn sites for enhanced CO hydrogenation. J. Am. Chem. Soc. 2025,147 (7), 5703–5713.
8. Li, Y.; Chen, K.; Yu, X.; Huang, W.; Ling, Y.; Shao, W.; Yang, F.*, Interface-Controlled Synthesis of Single-Ce and CeOx Catalysts on Copper Oxide Surfaces. ChemCatChem 2025,17 (18), e00609.
9. Lai, Y.; Chen, X.; Ma, Y.; Yan, W.; Meng, X.; Yang, F.*; Xiao, F.-S., Selective catalytic reduction of NOx with methane over Co-SSZ-16. Materials Today Nano 2025, 100725.
10. Lai, Y.; Chen, X.; Li, J.; Yan, W.; Meng, X.; Yang, F.; Xiao, F.-S., Efficient NOx abatement by passive adsorption over SSZ-16 zeolite supported palladium. Catal. Today 2025,455, 115314.
11. Guo, P.; Huang, Y.; Jin, C.; Zhou, D.; Han, S.; Zhou, Y.; Yang, F.; Shen, W., Active Pt Thin Layers over MoC for the Low-Temperature Water-Gas Shift Reaction. EES Catalysis 2025. DOI: 10.1039/d5ey00243e
12. Chen, Y.; Kong, X.; Yang, C.; Liao, Y.; Gao, G.; Ma, R.; Peng, M.; Shao, W.; Zheng, H.; Zhang, H.; Pan, X.; Yang, F.; Zhu, Y.; Liu, Z.; Cao, Y.; Ma, D.; Bao, X.; Zhu, Y., A catalytic cycle that enables crude hydrogen separation, storage and transportation. Nat. Energy 2025,10, 971–980.
13. Zhu, B.; Huang, W.; Lin, H.; Feng, H.; Palotás, K.; Lv, J.; Ren, Y.; Ouyang, R.*; Yang, F.*, Vacancy ordering in ultrathin copper oxide films on Cu(111). J. Am. Chem. Soc. 2024,146 (23), 15887-15896.
14. Shao, W.; Zhang, Y.; Zhou, Z.; Li, N.; Jiao, F.; Ling, Y.; Li, Y.; Zhou, Z.; Cao, Y.; Liu, Z.; Pan, X.; Fu, Q.; Wöll, C.; Liu, P.; Bao, X.; Yang, F.*, Dynamic control and quantification of active sites on ceria for CO activation and hydrogenation. Nat. Commun. 2024,15 (1), 9620.
15. Deng, X.; Zheng, C.; Li, Y.; Zhou, Z.; Wang, J.; Ran, Y.; Hu, Z.*; Yang, F.*; Li, L.*, Conductive catalysis by subsurface transition metals. Nat. Sci. Rev. 2024,11 (1), nwae015.
16. Zhou, Q.; Zhou, Z.; Lu, S.; Wang, L.; Zhan, X.; Peng, H.; Cai, J.; Wang, B.; Han, Y.; Zhao, A.; Tang, S.; Yang, F.*; Liu, Z.*, Increasing reactivity of ceria through water assisted surface modification. Appl. Surf. Sci. 2024,656, 159666.
17. Zhang, H.; Zhang, H.; Wang, R.; Lv, J.; Huang, W.; Guo, C.; Yang, F.*, Enhancing oxygen evolution reaction with two-dimensional nickel oxide on Au (111). Catalysts 2024,14 (5), 284.
18. Li, J.; Zhang, L.; Ma, Y.; Fan, K.; Zhang, J.; Wu, J.; Yan, W.; Meng, X.*; Wu, Q.; Yang, F.*; Xiao, F.-S.*, Selective catalytic reduction of NOx with methane over cobalt-exchanged SSZ-39 zeolite. Chem. Eng. J. 2024,496, 153191.
19. Wang, Y.-Q.; Fu, J.; Feng, Y.; Zhao, K.; Wang, L.; Cai, J.-Y.; Wang, X.; Chen, T.; Yang, F.; Hu, J.-S.; Xu, B.; Wang, D.*; Wan, L.-J.*, Alkali metal cations induce structural evolution on Au(111) during cathodic polarization. J. Am. Chem. Soc.2024,146 (40), 27713-27724.
20. Wang, M.; Zheng, L.; Wang, G.; Cui, J.; Guan, G.-L.; Miao, Y.-T.; Wu, J.-F.; Gao, P.; Yang, F.; Ling, Y.; Luo, X.; Zhang, Q.; Fu, G.; Cheng, K.; Wang, Y.*, Spinel nanostructures for the hydrogenation of CO2 to methanol and hydrocarbon chemicals. J. Am. Chem. Soc.2024,146 (21), 14528-14538.
21. Yang, C.; Ma, S.; Liu, Y.; Wang, L.; Yuan, D.; Shao, W.-P.; Zhang, L.; Yang, F.; Lin, T.; Ding, H.; He, H.; Liu, Z.-P.; Cao, Y.; Zhu, Y.*; Bao, X.*, Homolytic H2 dissociation for enhanced hydrogenation catalysis on oxides. Nat. Commun.2024,15 (1), 540.
22. Li, X.; Xu, Z.; Bu, D.; Cai, J.; Chen, H.; Chen, Q.; Chen, T.; Cheng, F.; Chi, L.; Dong, W.; Dong, Z.; Du, S.; Fan, Q.; Fan, X.; Fu, Q.; Gao, S.; Guo, J.; Guo, W.; He, Y.; Hou, S.; Jiang, Y.; Kong, H.; Li, B.; Li, D.; Li, J.; Li, Q.; Li, R.; Li, S.; Lin, Y.; Liu, M.; Liu, P.; Liu, Y.; Lü, J.; Ma, C.; Pan, H.; Pan, J.; Pan, M.; Qiu, X.; Shen, Z.; Tan, S.; Wang, B.; Wang, D.; Wang, L.; Wang, L.; Wang, T.; Wang, X.; Wang, X.; Wang, X.; Wang, Y.; Wang, Y.; Wu, K.; Xu, W.; Xue, N.; Yan, L.; Yang, F.; Yang, Z.; Zhang, C.; Zhang, X.; Zhang, Y.; Zhang, Y.; Zhou, X.; Zhu, J.; Zhang, Y.; Gao, F.*; Wang, Y.*, Recent progress on surface chemistry II: Property and characterization. Chin. Chem. Lett.2024,36 (1), 110100.
23. Li, X.; Xu, Z.; Bu, D.; Cai, J.; Chen, H.; Chen, Q.; Chen, T.; Cheng, F.; Chi, L.; Dong, W.; Dong, Z.; Du, S.; Fan, Q.; Fan, X.; Fu, Q.; Gao, S.; Guo, J.; Guo, W.; He, Y.; Hou, S.; Jiang, Y.; Kong, H.; Li, B.; Li, D.; Li, J.; Li, Q.; Li, R.; Li, S.; Lin, Y.; Liu, M.; Liu, P.; Liu, Y.; Lü, J.; Ma, C.; Pan, H.; Pan, J.; Pan, M.; Qiu, X.; Shen, Z.; Tan, S.; Wang, B.; Wang, D.; Wang, L.; Wang, L.; Wang, T.; Wang, X.; Wang, X.; Wang, X.; Wang, Y.; Wang, Y.; Wu, K.; Xu, W.; Xue, N.; Yan, L.; Yang, F.; Yang, Z.; Zhang, C.; Zhang, X.; Zhang, Y.; Zhang, Y.; Zhou, X.; Zhu, J.; Zhang, Y.; Gao, F.*; Wang, Y.*, Recent progress on surface chemistry I: Assembly and reaction. Chin. Chem. Lett.2024,35 (12), 110055.
24. Zhao, S.; Fan, K.; Li, J.; Ma, Y.; Yang, F.; Meng, X.; Xiao, F.-S.*, Hydrophobic modification of zeolite-supported platinum catalysts for complete oxidation of toluene. Catal. Today2024,432, 114601.
25. Lan, Y.; Wang, L.; Luo, Y.; Hao, R.; Zhang, H.; Aruta, C.; Yang, F.; Yu, Y.; Yang, N.*, Engineering lanthanum into Pt doped CeO2 for Intermediate temperature solid oxide fuel cells. J. Eur. Ceram. Soc.2024,44 (2), 996-1004.
26. Fei, Y.; Yang, W.; Guo, Z.; Sun, H.; Yang, F.; Hu, J.*, Study of cell adhesion, osteogenesis, and angiogenesis of a “groove” structure micro-arc oxidation titanium. Applied Surface Science Advances2024,19, 100552.
27. Ding, B.; Yang, C.; Chen, Y.; Shao, W.-P.; Yang, F.; Zhang, C.; Wang, Z.; Liu, Y.; Cao, Y.; Zhu, Y.*; Bao, X.*, Cr2O3 clusters on ZnO as hydrogen pools for efficient syngas‐to‐light olefins. ChemCatChem2024,16 (23), e202401421.
28. Zhang, Y.; Li, H.; Liu, F.; Li, M.; Zhang, Y.; Cai, J.; Li, Y.; Yang, F.; Yin, F.; Lu, J.; Zhang, T.; Yang, B.*, Revealing dynamics and competitive mechanism of gas-induced surface segregation of PdFe0.08 dilute alloy by multi-dimensional imaging. J. Phys. Chem. Lett.2024,15 (47), 11737-11744.
29. Chen, Z.; Wen, J.; Zeng, Y.; Li, M.; Tian, Y.; Yang, F.; Li, M. M.-J.; Chen, P.; Huang, H.; Ye, D.; Chen, L.*, The origin of the mediocre methanol selectivity of Cu/ZnO-based catalysts for methanol synthesis from CO2 hydrogenation. Appl. Catal. B2024,340, 123192.
30. Ling, Y.; Luo, J.; Ran, Y.; Liu, Z.; Li, W.-X.; Yang, F.*, Atomic-scale visualization of heterolytic H2 dissociation and COx hydrogenation on ZnO under ambient conditions. J. Am. Chem. Soc.2023,145 (41), 22697-22707.
31. Zhou, Z.; Chen, L.; Wang, L.; Liu, Y.; Cheng, P.; Peng, H.; Cai, J.; Zhou, Q.; Wang, Y.; Yang, N.; Wang, B.; Gong, X.-Q.; Yang, F.*; Liu, Z.*, Selective hydrogenation of propyne to propene promoted by synergistic effect of surface oxygen vacancies and hydride species on Ceria. ACS Catal.2023,13 (14), 9588-9596.
32. Wang, X.; Guo, C.; Zhu, B.; Xiao, D.; Gao, D.; Liu, Z.; Yang, F.*, Reaction-induced iodine adsorption on Cu surfaces facilitates electrocatalytic CO2 reduction. J. Chem. Phys.2023,158 (20), 204701.
33. Zhao, L.; Zhang, L.; Wu, Z.; Huang, C.; Chen, K.; Wang, H.; Yang, F.*, Size effect of Cu particles on interface formation in Cu/ZnO catalysts for methanol synthesis. Catalysts2023,13 (8), 1190.
34. Zhou, Q.; Akber, H.; Zhao, A.; Yang, F.*; Liu, Z.*, Interaction of water with ceria thin film. ChemCatChem2023,15 (15), e2023003.
35. Cai, J.; Ling, Y.; Zhang, H.; Yang, B.; Yang, F.*; Liu, Z.*, Formation of different Rh–O species on Rh(110) and their reaction with CO. ACS Catal.2023,13 (1), 11-18.
36. Zang, Y.; Cai, J.; Han, Y.; Wu, H.; Zhu, W.; Shi, S.; Zhang, H.; Ran, Y.; Yang, F.; Ye, M.; Yang, B.; Li, Y.; Liu, Z.*, CO2 activation on Ni(111) and Ni(110) surfaces in the presence of hydrogen. J. Phys. Chem. Lett.2023,14 (19), 4381-4387.
37. Li, Z.; Chen, L.; Wu, Z.; Jia, A.; Shi, S.; Zhang, H.; Wang, J.; Liu, Z.; Shao, W.-P.; Yang, F.; Wu, X.-P.; Gong, X.-Q.; Huang, W.*, Surface oxygen vacancy and hydride species on Ceria are detrimental to acetylene semihydrogenation reaction. ACS Catal.2023,13 (8), 5213-5224.
38. Wu, M.-Y.; Wang, B.-B.; Wang, W.-W.; Yang, F.; Jia, C.-J.*, Dynamic structural evolution of CeO2 in CuO−CeO2 catalyst revealed by in situ spectroscopy. ChemCatChem2023,15 (22), e202300894.
39. Liu, Q.; Li, Y.; Zhao, X.; Zhu, B.; Yi, Z.; Yang, F.*; Bao, X., Dynamic structural changes of iron oxide nanostructures on Cu(111). J. Phys. Chem. C2022,126 (4), 2041-2048.
40. Liu, K.; Jiang, L.; Huang, W.; Zhu, G.; Zhang, Y.-J.; Xu, C.; Qin, R.; Liu, P.; Hu, C.; Wang, J.; Li, J.-F.; Yang, F.*; Fu, G.*; Zheng, N.*, Atomic overlayer of permeable microporous cuprous oxide on palladium promotes hydrogenation catalysis. Nat. Commun.2022,13 (1), 2597.
41. Ling, Y.; Ran, Y.; Shao, W.; Li, N.; Jiao, F.; Pan, X.; Fu, Q.; Liu, Z.; Yang, F.*; Bao, X., Probing active species for CO hydrogenation over ZnCr2O4 catalysts. Chin. J. Catal.2022,43 (8), 2017-2025.
42. Ling, Y.; Luo, J.; Ran, Y.; Cao, Y.; Huang, W.; Cai, J.; Liu, Z.; Li, W.-X.*; Yang, F.*; Bao, X., Dynamic chemical processes on ZnO surfaces tuned by physisorption under ambient conditions. J. Energy Chem.2022,72, 258-264.
43. Su, X.; Jiang, Z.; Zhou, J.; Liu, H.; Zhou, D.; Shang, H.; Ni, X.; Peng, Z.; Yang, F.; Chen, W.; Qi, Z.; Wang, D.; Wang, Y.*, Complementary Operando Spectroscopy identification of in-situ generated metastable charge-asymmetry Cu2-CuN3 clusters for CO2 reduction to ethanol. Nat. Commun.2022,13 (1), 1322.
44. Sang, J.; Wei, P.; Liu, T.; Lv, H.; Ni, X.; Gao, D.; Zhang, J.; Li, H.; Zang, Y.; Yang, F.; Liu, Z.; Wang, G.*; Bao, X.*, A reconstructed Cu2P2O7 catalyst for selective CO2 electroreduction to multicarbon products. Angew. Chem. Int. Ed.2022,61 (5), e202114238.
45. Xu, W.; Ni, X.; Zhang, L.; Yang, F.; Peng, Z.; Huang, Y.; Liu, Z.*, Tuning the electronic structure of tungsten oxide for enhanced hydrogen evolution reaction in alkaline electrolyte. ChemElectroChem2022,9 (5), e202101300.
46. Mao, Z.; Ding, C.; Liu, X.; Zhang, Q.; Qin, X.; Li, H.; Yang, F.; Li, Q.; Zhang, X.-G.; Zhang, J.; Cai, W.-B.*, Interstitial B-doping in Pt lattice to upgrade oxygen electroreduction performance. ACS Catal.2022,12 (15), 8848-8856.
47. Zhan, X.; Luo, Y.; Wang, Z.; Xiang, Y.; Peng, Z.; Han, Y.; Zhang, H.; Chen, R.; Zhou, Q.; Peng, H.; Huang, H.; Liu, W.; Ou, X.; Ma, G.; Fan, F.; Yang, F.; Li, C.; Liu, Z.*, Formation of multifaceted nano-groove structure on rutile TiO2 photoanode for efficient electron-hole separation and water splitting. J. Energy Chem.2022,65, 19-25.
48. Li, X.; Zhang, H.; Ran, Y.; Ye, M.; Yang, F.; Han, Y.; Liu, Z.*, Beam-induced effects on platinum oxidation during ambient-pressure X-ray photoelectron spectroscopy. J. Phys. Chem. Lett.2022,13 (24), 5677-5682.
49. Jin, C.; Wang, B.; Zhou, Y.*; Yang, F.*; Han, S.; Guo, P.; Liu, Z.; Shen, W.*, Gold atomic layers and isolated atoms on MoC for the low-temperature water gas shift reaction. ACS Catal.2022,12 (24), 15648-15657.
50. Jin, C.; Wang, B.; Zhou, Y.*; Yang, F.*; Guo, P.; Liu, Z.; Shen, W.*, Restructuring of the gold-carbide interface for low-temperature water-gas shift. Chem. Comm.2022,58 (52), 7313-7316.
51. Huang, W.*; Yang, F.*, Preface to special column on surface & interface chemistry connecting thermo-, photo- and electro-catalysis. Chin. J. Catal.2022,43 (8), 1963.
52. Dong, A.; Lin, L.; Mu, R.; Li, R.; Li, K.; Wang, C.; Cao, Y.; Ling, Y.; Chen, Y.; Yang, F.; Pan, X.; Fu, Q.*; Bao, X.*, Modulating the formation and evolution of surface hydrogen species on ZnO through Cr addition. ACS Catal.2022,12 (10), 6255-6264.
53. Zhou, Q.; Cai, J.; Wang, W.; Liu, Z.*; Yang, F.*, In-situ studies of catalytic reactions over well-defined model catalysts. In Catal., The Royal Society of Chemistry: Cambridge, 2021; Vol. 33, pp 380-416.
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